Publications

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2017

  1. A. Moreno, S. Grama, T. Liu, M. Galia, G. Lligadas & V. Percec. SET-LRP Mediated by TREN in Biphasic Water-Organic Solvent Mixtures Provides the Most Economical and Efficient Process. Polym. Chem. 2017, 8, 7559-7574.
    DOI: 10.1039/c7py01841j.
  2. J. Kopitz, Q. Xiao, A.-K. Ludwig, A. Romero, M. Michalak, S. E. Sherman, X. Zhou, C. Dazen, S. Vertesy, H. Kaltner, M. L. Klein, H.-J. Gabius & V. Percec. Reaction of a Programmable Glycan Presentation of Glycodendrimersomes and Cells with Engineered Human Lectins To Show the Sugar Functionality of the Cell Surface. Angew. Chem. Int. Ed. 2017, 56, 14677–14681.
    DOI: 10.1002/anie.201708237.
  3. G. Lligadas, S. Grama & V. Percec. SET-LRP Platform to Practice, Develop and Invent. Biomacromolecules 2017, 18, 2981-3008.
    DOI: 10.1021/acs.biomac.7b01131.
  4. A. Moreno, D. Garcia, M. Galia, J. C. Ronda, V. Cadiz, G. Lligadas & V. Percec. SET-LRP in the Neoteric Ethyl Lactate Alcohol. Biomacromolecules 2017, 18, 3447-3456.
    DOI: 10.1021/acs.biomac.7b01130
  5. S. Grama, J. E. Lejnieks, M. Enayati, R. B. Smail, L. Ding, G. Lligadas, M. J. Monteiro & V. Percec. Searching for Efficient SET-LRP Systems via Biphasic Mixtures of Water with Carbonates, Ethers and Dipolar Aprotic Solvents. Polym. Chem. 2017, 8, 5865-5874.
    DOI: 10.1039/c7py01349c.
  6. K. A. Andreopoulou, M. Peterca, D. A. Wilson, B. E. Partridge, P. A. Heiney & V. Percec. Demonstrating the 81-Helicity and Nanomechanical Function of Self-Organizable Dendronized Polymethacrylates and Polyacrylates. Macromolecules 2017, 50, 5271-5284.
    DOI: 10.1021/acs.macromol.7b01216.
  7. G. Lligadas, M. Enayati, S. Grama, R. Smail, S. E. Sherman & V. Percec. Ultrafast SET-LRP with Peptoid Cytostatic Drugs as Monofunctional and Bifunctional Initiators. Biomacromolecules 2017, 18, 2610-2622.
    DOI: 10.1021/acs.biomac.7b00722.
  8. Q. Xiao, S. E. Sherman, S. E. Wilner, X. Zhou, C. Dazen, T. Baumgart, E. H. Reed, D. A. Hammer, W. Shinoda, M. L. Klein & V. Percec. Janus Dendrimersomes Coassembled from Fluorinated, Hydrogenated and Hybrid Janus Dendrimers as Models for Fusion and Fission of Biological Cells. Proc. Natl. Acad. Sci. U.S.A. 2017, 114, E7045-E7053.
    DOI: 10.1073/pnas.1708380114.
  9. R. L. Jezorek, M. Enayati, R. B. Smail, J. Lejnieks, S. Grama, M. J. Monteiro & V. Percec. The Stirring Rate Provides A Dramatic Acceleration of the Ultrafast Interfacial SET-LRP in Biphasic Acetonitrile-Water Mixtures. Polym. Chem. 2017, 8, 3405-3424.
    DOI: 10.1039/c7py00659d.
    Featured on Front Cover of the issue.
  10. R. B. Smail, R. L. Jezorek, J. Lejnieks, M. Enayati, S. Grama, M. J. Monteiro & V. Percec. Acetone-Water Biphasic Mixtures as Solvents for Ultrafast SET-LRP of Hydrophobic Acrylates. Polym. Chem. 2017, 8, 3102-3123.
    DOI: 10.1039/c7py00557a.
  11. S. E. Sherman, Q. Xiao & V. Percec. Mimicking Complex Biological Membranes and Their Programmable Glycan Ligands with Dendrimersomes and Glycodendrimersomes. Chem. Rev. 2017, 117, 6538-6631.
    DOI: 10.1021/acs.chemrev.7b00097.
  12. G. Lligadas, S. Grama & V. Percec. Recent Developments in the Synthesis of Biomacromolecules and Their Conjugates by SET-LRP. Biomacromolecules 2017, 18, 1039-1063.
    DOI: 10.1021/acs.biomac.7b00197.
    Selected as ACS Editors’ Choice and featured on the Front Cover of the issue.
  13. D. Jishkariani, C. M. MacDermaid, Y. N. Timsina, S. Grama, S. S. Gillani, M. Divar, S. S. Yadavalli, R.-O. Moussodia, P. Leowanawat, A. M. Berrios Camacho, R. Walter, M. Goulian, M. L. Klein & V. Percec. Self-Interrupted Synthesis of Sterically Hindered Aliphatic Polyamide Dendrimers. Proc. Natl. Acad. Sci. U.S.A. 2017, 114, E2275-E2284.
    DOI: 10.1073/pnas.1700922114.
    Highlighted by Ali Sundermier on Penn News.
  14. D. Sahoo, M. Peterca, E. Aqad, B. E. Partridge, P. A. Heiney, R. Graf, H. W. Spiess, X. Zeng & V. Percec. Tetrahedral Arrangements of Perylene Bisimide Columns via Supramolecular Orientational Memory. ACS Nano 2017, 11, 983-991.
    DOI: 10.1021/acsnano.6b07599.
  15. M. N. Holerca, D. Sahoo, M. Peterca, B. E. Partridge, P. A. Heiney & V. Percec. A Tetragonal Phase Self-Organized from Unimolecular Spheres Assembled from a Substituted Poly(2-oxazoline). Macromolecules 2017, 50, 375-385.
    DOI: 10.1021/acs.macromol.6b02298.
  16. 2016

  17. M. Enayati, R. B. Smail, S. Grama, R. L. Jezorek, M. L. Monteiro & V. Percec. The Synergistic Effect During Biphasic SET-LRP in Ethanol-Nonpolar Solvent-Water Mixtures. Polym. Chem. 2016, 7, 7230-7241.
    DOI: 10.1039/c6py01815g.
  18. M. Vorobii, O. Pop-Georgievski, A. de los Santos Pereira, N. Yu. Kostina, R. L. Jezorek, Z. Sedlakova, V. Percec & C. Rodriguez-Emmenegger. Grafting of Functional Methacrylate Polymer Brushes by Photoinduced SET-LRP. Polym. Chem. 2016, 7, 6934-6945.
    DOI: 10.1039/c6py01730d.
  19. D. Sahoo, M. Peterca, E. Aqad, B. E. Partridge, P. A. Heiney, R. Graf, H. W. Spiess, X. Zeng & V. Percec. Hierarchical Self-Organization of Perylene Bisimides into Supramolecular Spheres and Periodic Arrays Thereof. J. Am. Chem. Soc. 2016, 138, 14798-14807.
    DOI: 10.1021/jacs.6b09986.
  20. M. Peterca, M. R. Imam, S. D. Hudson, B. E. Partridge, D. Sahoo, P. A. Heiney, M. L. Klein & V. Percec. Complex Arrangement of Orthogonal Nanoscale Columns via a Supramolecular Orientational Memory Effect. ACS Nano 2016, 10, 10480-10488.
    DOI: 10.1021/acsnano.6b06419.
  21. M.-S. Ho, B. E. Partridge, H.-J. Sun, D. Sahoo, P. Leowanawat, M. Peterca, R. Graf, H. W. Spiess, X. Zeng, G. Ungar, P.A. Heiney, C.-S. Hsu & V. Percec. Screening Libraries of Semifluorinated Arylene Bisimides to Discover and Predict Thermodynamically Controlled Helical Crystallization. ACS Comb. Sci. 2016, 18, 723-739.
    DOI: 10.1021/acscombsci.6b00143.
    Front Cover of the Issue.
  22. Q. Xiao, Z. Wang, D. Williams, P. Leowanawat, M. Peterca, S. E. Sherman, S. Zhang, D. A. Hammer, P. A. Heiney, S. R. King, D. M. Markovitz, S. Andre, H.-J. Gabius, M. L. Klein & V. Percec. Why Do Membranes of Some Unhealthy Cells Adopt a Cubic Architecture? ACS Cent. Sci. 2016, 2, 943-953.
    DOI: 10.1021/acscentsci.6b00284.
    Highlighted by Ali Sundermier on Penn News.
  23. Q. Xiao, J. D. Rubien, Z. Wang, E. H. Reed, D. A. Hammer, D. Sahoo, P. A. Heiney, S. S. Yadavalli, M. Goulian, S. E. Wilner, T. Baumgart, S. A. Vinogradov, M. L. Klein & V. Percec. Self-Sorting and Coassembly of Fluorinated, Hydrogenated, and Hybrid Janus Dendrimers into Dendrimersomes. J. Am. Chem. Soc. 2016, 138, 12655-12663.
    DOI: 10.1021/jacs.6b08069.
  24. M. Enayati, R. L. Jezorek, R. B. Smail, M. J. Monteiro & V. Percec. Ultrafast SET-LRP in Biphasic Mixtures of the Non-Disproportionating Solvent Acetonitrile with Water. Polym. Chem. 2016, 7, 5930-5942.
    DOI: 10.1039/c6py01307d.
  25. M. Gavrilov, Z. Jia, V. Percec & M. J. Monteiro. Quantitative End-Group Functionalization of PNIPAM from Aqueous SET-LRP via in situ Reduction of Cu(II) with NaBH4. Polym. Chem. 2016, 7, 4802-4809.
    DOI: 10.1039/c6py00968a.
    Selected by Dr. Athina Anastasaki as Polymer Chemistry‘s Paper of the Month.
  26. M. Enayati, R. L. Jezorek & V. Percec. A Multiple-Stage Activation of the Catalytically Inhomogeneous Cu(0) Wire Used in SET-LRP. Polym. Chem. 2016, 7, 4549-4558.
    DOI: 10.1039/c6py00888g.
  27. J. Malineni, R. L. Jezorek, N. Zhang & V. Percec. NiIICl(1-Naphthyl)(PCy3)2, an Air-Stable σ-NiII Precatalyst for Quantitative Cross-Coupling of Aryl C-O Electrophiles with Aryl Neopentylglycolboronates. Synthesis 2016, 48, 2808-2815.
    DOI: 10.1055/s-0035-1562343.
  28. J. Malineni, R. L. Jezorek, N. Zhang & V. Percec. “An Indefinitely Air-Stable σ-NiII Precatalyst for Quantitative Cross-Coupling of Unreactive Aryl Halides and Mesylates with Aryl Neopentylglycolboronates. Synthesis 2016, 48, 2795-2807.
    DOI: 10.1055/s-0035-1562342.
  29. M. Enayati, R. L. Jezorek, M. J. Monteiro & V. Percec. Ultrafast SET-LRP of Hydrophobic Acrylates in Multiphase Alcohol-Water Mixtures. Polym. Chem. 2016, 7, 3608-3621.
    DOI: 10.1039/C6PY00353B.
  30. Q. Xiao, S. S. Yadavalli, S. Zhang, S. E. Sherman, E. Fiorin, L. da Silva, D. A. Wilson, D. A. Hammer, S. André, H.-J. Gabius, M. L. Klein, M. Goulian & V. Percec. Bioactive Cell-Like Hybrids Coassembled from (Glyco)Dendrimersomes with Bacterial Membranes. Proc. Natl. Acad. Sci. U.S.A. 2016, 113, E1134-E1141.
    DOI: 10.1073/pnas.1525589113.
  31. V. Percec. Introduction to Frontiers in Macromolecular and Supramolecular Science: Part 2. Chem. Rev. 2016, 116, 1671-1672.
    DOI: 10.1021/acs.chemrev.6b00069.
  32. V. Percec. Introduction to Frontiers in Macromolecular and Supramolecular Science: Part 1. Chem. Rev. 2016, 116, 769-770.
    DOI: 10.1021/acs.chemrev.6b00058.
  33. M. Gavrilov, T. J. Zerk, P. V. Bernhardt, V. Percec & M. J. Monteiro. SET-LRP of NIPAM in Water via in situ Reduction of Cu(II) to Cu(0) with NaBH4. Polym. Chem. 2016, 7, 406-417.
    DOI: 10.1039/C5PY01855B.
  34. Q. Xiao, S. Zhang, Z. Wang, S. E. Sherman, R.-O. Moussodia, M. Peterca, A. Muncan, D. R. Williams, D. A. Hammer, S. Vértesy, S. André, H.-J. Gabius, M. L. Klein & V. Percec. Onion-Like Glycodendrimersomes from Sequence-Defined Janus Glycodendrimers and Influence of Architecture on Reactivity to a Lectin. Proc. Natl. Acad. Sci. U.S.A. 2016, 113, 1162-1167.
    DOI: 10.1073/pnas.1524976113.
  35. C. Roche, H.-J. Sun, P. Leowanawat, F. Araoka, B. E. Partridge, M. Peterca, D. A. Wilson, M. E. Prendergast, P. A. Heiney, R. Graf, H. W. Spiess, X. Zeng, G. Ungar & V. Percec. A Supramolecular Helix that Disregards Chirality. Nat. Chem. 2016, 8, 80-89.
    DOI: 10.1038/NCHEM.2397.
    Highlighted by S. Borman, “How Researchers Formed A Pure, Chiral Crystal From Mixed Ingredients” in Chem. Eng. News 2015, 93 (48), 9.
  36. 2015

  37. S. Zhang, Q. Xiao, S. E. Sherman, A. Muncan, A. D. M. Ramos Vicente, Z. Wang, D. A. Hammer, D. Williams, Y. Chen, D. J. Pochan, S. Vértesy, S. André, M. L. Klein, H.-J. Gabius & V. Percec. Glycodendrimersomes from Sequence-Defined Janus Glycodendrimers Reveal High Activity and Sensor Capacity for the Agglutination by Natural Variants of Human Lectins. J. Am. Chem. Soc. 2015, 137, 13334-13344.
    DOI: 10.1021/jacs.5b08844.
    Spotlight by R. Mukhopadhyay, “Clarifying Sugar-Receptor Binding” in J. Am. Chem. Soc. 2015, 137, 13211. DOI: 10.1021/jacs.5b10594.
  38. O. V. Kulikov, D. A. Siriwardane, J. F. Reuther, G. T. McCandless, H.-J. Sun, Y. Li, S. F. Mahmood, S. S. Sheiko, V. Percec & B. M. Novak. Characterization of Fibrous Aggregated Morphologies and Other Complex Architectures Self-Assembled from Helical Alkyne and Triazole Polycarbodiimides (R)- and (S)-Families in the Bulk and Thin Film. Macromolecules 2015, 48, 4088-4103.
    DOI: 10.1021/acs.macromol.5b00407.
  39. M. Vorobii, A. de Los Santos Pereira, O. Pop-Georgievski, N. Yu. Kostina, C. Rodriguez-Emmenegger & V. Percec. Synthesis of Non-Fouling Poly[N-(2-hydroxypropyl)methacrylamide] Brushes by Photoinduced SET-LRP. Polym. Chem. 2015, 6, 4210-4220.
    DOI: 10.1039/c5py00506j.
  40. S. Zhang, R.-O. Moussodia, S. Vértesy, S. André, M. L. Klein, H.-J. Gabius & V. Percec. Unraveling Functional Significance of Natural Variations of a Human Galectin by Glycodendrimersomes with Programmable Glycan Surface. Proc. Natl. Acad. Sci. U.S.A. 2015, 112, 5585-5590.
    DOI: 10.1073/pnas.1506220112.
  41. B. E. Partridge, P. Leowanawat, E. Aqad, M. R. Imam, H.-J. Sun, M. Peterca, P. A. Heiney, R. Graf, H. W. Spiess, X. Zeng, G. Ungar & V. Percec. Increasing 3D Supramolecular Order by Decreasing Molecular Order. A Comparative Study of Helical Assemblies of Dendronized Nonchlorinated and Tetrachlorinated Perylene Bisimides. J. Am. Chem. Soc. 2015, 137, 5210-5224.
    DOI: 10.1021/jacs.5b02147.
    Spotlight by C. Herman, “An Unexpected Finding About Highly Ordered Supramolecular Assemblies” in J. Am. Chem. Soc. 2015, 137, 4875. DOI: 10.1021/jacs.5b03817.
  42. S. Guerra, J. Iehl, M. Holler, M. Peterca, D. A. Wilson, B. E. Partridge, S. Zhang, R. Deschenaux, J.-F. Nierengarten & V. Percec. Self-Organisation of Dodeca-Dendronized Fullerene into Supramolecular Discs and Helical Columns Containing a Nanowire-Like Core. Chem. Sci. 2015, 6, 3393-3401.
    DOI: 10.1039/c5sc00449g.
  43. S. R. Samanta, R. Cai & V. Percec. A Rational Approach to Activated Polyacrylates and Polymethacrylates by Using a Combination of Model Reactions and SET-LRP of Hexafluoroisopropyl Acrylate and Methacrylate. Polym. Chem. 2015, 6, 3259-3270.
    DOI: 10.1039/C5py00082C.
  44. S. R. Samanta, V. Nikolaou, S. Keller, M. J. Monteiro, D. A. Wilson, D. M. Haddleton & V. Percec. Aqueous SET-LRP Catalyzed with “in situ” Generated Cu(0) Demonstrates Surface Mediated Activation and Bimolecular Termination. Polym. Chem. 2015, 6, 2084-2097.
    DOI: 10.1039/c4py01748j.
  45. R. Zhang, X. Zeng, B. Kim, R. J. Bushby, K. Shin, P. J. Baker, V. Percec, P. Leowanawat & G. Ungar. Columnar Liquid Crystals with Cylindrical Nanoconfinement. ACS Nano 2015, 9, 1759-1766.
    DOI: 10.1021/nn506605p.
  46. S. Zhang, R.-O. Moussodia, C. Murzeau, H.-J. Sun, M. L. Klein, S. Vértesy, S. André, R. Roy, H.-J. Gabius & V. Percec. Dissecting Molecular Aspects of Cell Interactions Using Glycodendrimersomes with Programmable Glycan Presentation and Engineered Human Lectins. Angew. Chem. Int. Ed. 2015, 54, 4036-4040.
    DOI: 10.1002/anie.201410882.
  47. Y.-C. Wu, P. Leowanawat, H.-J. Sun, B. E. Partridge, M. Peterca, R. Graf, H. W. Spiess, X. Zeng, G. Ungar, C.S. Hsu, P. A. Heiney & V. Percec. Complex Columnar Hexagonal Polymorphism in Supramolecular Assemblies of a Semifluorinated Electron-Accepting Naphthalene Bisimide. J. Am. Chem. Soc. 2015, 137, 807-819.
    DOI: 10.1021/ja510643b.
  48. H.-J. Sun, S. Zhang & V. Percec. From Structure to Function via Complex Supramolecular Dendrimer Systems. Chem. Soc. Rev. 2015, 44, 3900-3923.
    DOI: 10.1039/c4cs00249k.
  49. S. R. Samanta, R. Cai & V. Percec. Synthesis of Amphiphilic Homopolymers with High Chain End Functionality by SET-LRP. J. Polym. Sci.: Part A, Polym. Chem. 2015, 53, 294-303.
    DOI: 10.1002/pola.27331.
  50. 2014

  51. R. L. Jezorek, N. Zhang, P. Leowanawat, M. H. Bunner, N. Gutsche, A. K. R. Pesti, J. T. Olsen & V. Percec. Air- Stable Precatalysts for Fast and Quantitative Cross-Coupling of Aryl Sulfamates with Arylneopentylglycolboronates at Room Temperature. Org. Lett. 2014, 16, 6326-6329.
    DOI: 10.1021/ol503061c.
  52. S. R. Samanta, R. Cai & V. Percec. SET-LRP of Semifluorinated Acrylates and Methacrylates. Polym. Chem. 2014, 5, 5479-5491.
    DOI: 10.1039/c4py00635f.
  53. C. Roche, H.-J. Sun, M. E. Prendergast, P. Leowanawat, B. E. Partridge, P. A. Heiney, F. Araoka, R. Graf, H. W. Spiess, X. Zeng, G. Ungar & V. Percec. Homochiral Columns Constructed by Chiral Self-Sorting During Supramolecular Helical Organization of Hat-Shaped Molecules. J. Am. Chem. Soc. 2014, 136, 7169-7185.
    DOI: 10.1021/ja5035107.
  54. S. Zhang, R.-O. Moussodia, H.-J. Sun, P. Leowanawat, A. Muncan, C. D. Nusbaum, K. M. Chelling, P. A. Heiney, M. L. Klein, S. André, R. Roy, H.-J. Gabius & V. Percec. Mimicking Biological Membranes with Programmable Glycan Ligands Self-Assembled from Amphiphilic Janus Glycodendrimers. Angew. Chem. Int. Ed. 2014, 53, 10899-10903.
    DOI: 10.1002/anie.201403186.
  55. S. Zhang, H.-J. Sun, A. D. Hughes, R.-O. Moussodia, A. Bertin, Y. Chen, D. J. Pochan, P. A. Heiney, M. L. Klein & V. Percec. Self-Assembly of Amphiphilic Janus Dendrimers into Uniform Onion-Like Dendrimersomes with Predictable Size and Number of Bilayers. Proc. Natl. Acad. Sci. U.S.A. 2014, 111, 9058-9063.
    DOI: 10.1073/pnas.1402858111.
    Highlighted by S. Borman, “Two Faced Dendrimers form Onionlike Vesicles” in Chem. Eng. News. 2014, 92 (25), 29.
  56. N. Zhang, S. R. Samanta, B. M. Rosen & V. Percec. Single Electron Transfer in Radical Ion and Radical-Mediated Organic, Materials and Polymer Synthesis. Chem. Rev. 2014, 114, 5848-5958.
    DOI: 10.1021/cr400689s.
  57. A. Anastasaki, V. Nikolaou, Q. Zhang, J. Burns, S. R. Samanta, C. Wandron, A. J. Haddleton, R. McHale, D. Fox, V. Percec, P. Wilson & D. M. Haddleton. Copper(II)/Tertiary Amine Synergy in Photoinduced Living Radical Polymerization: Accelerated Synthesis of ω-Functional and α,ω-Heterofunctional Poly(acrylates). J. Am. Chem. Soc. 2014, 136, 1141-1149.
    DOI: 10.1021/ja411780m.
  58. S. Zhang, H.-J. Sun, A. D. Hughes, B. Draghici, J. Lejnieks, P. Leowanawat, A. Bertin, L. O. De Leon, O. V. Kulikov, Y. Chen, D. J. Pochan, P. A. Heiney & V. Percec. “Single-Single” Amphiphilic Janus Dendrimers Self-Assemble into Uniform Dendrimersomes with Predictable Size. ACS Nano 2014, 8, 1554-1565.
    DO: 10.1021/nn405790x.
  59. S. R. Samanta & V. Percec. Synthesis of High Molar Mass Poly(N-Butyl Acrylate) and Poly(2-Ethylhexyl Acrylate) by SET-LRP in Mixtures of Fluorinated Alcohols with DMSO. Polym. Chem. 2014, 5, 169-174.
    DOI: 10.1039/c3py01008b.
  60. S. R. Samanta, H.-J. Sun, A. Anastasaki, D. M. Haddleton & V. Percec. Self-Activation and Activation of Cu(0) Wire for SET-LRP Mediated by Fluorinated Alcohols. Polym. Chem. 2014, 5, 89-95.
    DOI: 10.1039/c3py01007d.

Earlier

A full list of publications co-authored by Professor Percec can be viewed here.

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